Cast

• Sean Connery James Bond
• Daniela Bianchi Tatiana Romanova
• Pedro Armendáriz Ali Kerim Bey (as Pedro Armendariz)
• Lotte Lenya Rosa Klebb
• Robert Shaw Donovan 'Red' Grant
• Bernard Lee M
• Eunice Gayson Sylvia Trench
• Walter Gotell Morzeny
• Francis De Wolff Vavra, the Gypsy Leader (as Francis de Wolff)
• George Pastell Train Conductor
• Nadja Regin Kerim's Girl
• Lois Maxwell Miss Moneypenny
• Aliza Gur Vida
• Martine Beswick Zora (also as Martin Beswick)
• Vladek Sheybal Kronsteen
• Lisa Guiraut Gypsy Belly Dancer (as Leila)
• Hasan Ceylan Foreign Agent
• Fred Haggerty Krilencu
• Neville Jason Kerim's Chauffeur
• Peter Bayliss Benz
• Nusret Ataer Mehmet (as Nushet Ataer)
• Peter Brayham Rhoda
• Desmond Llewelyn Major Boothroyd
• Jan Williams Masseuse
• Peter Madden McAdams, Chess Player
• Dorothea Bennett Woman on Bridge in Venice (uncredited)
• Bedri Çavusoglu Police (uncredited)
• Elizabeth Counsell Woman in a Punt (uncredited)
• Michael Culver Man in a Punt (uncredited)
• Anthony Dawson Ernst Stavro Blofeld (uncredited)
• Moris Farhi Gypsy (uncredited)
• William Hill Captain Nash (uncredited) (as Bill Hill)
• Barbara Jefford Tatiana Romanova (voice) (uncredited)
• Muhammat Kohen Mosque Tour Guide (uncredited)
• Julie Mendez Girl dancing during opening titles (uncredited)
• Eric Pohlmann Ernst Stavro Blofeld (voice) (uncredited)
• Jaqi Saltzman Woman on train (uncredited)
• Bob Simmons James Bond in Gunbarrel Sequence (uncredited)
• Nikki Van der Zyl Receptionist (voice) (uncredited)

Writers

• Ian Fleming
• Johanna Harwood
• Richard Maibaum

Producers

• Albert R. Broccoli
• Harry Saltzman
• Stanley Sopel